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1910–1920

In 1910 Bunin published The Village (Деревня), a bleak portrayal of Russian country life, which he depicted as full of stupidity, brutality, and violence. This book caused controversy and made him famous. Its harsh realism (with "characters having sunk so far below the average level of intelligence as to be scarcely human") prompted Maxim Gorky to call Bunin "the best Russian writer of the day."

"I've left behind my "narodnicism" which didn't last very long, my Tolstoyism too and now I'm closer to the social democrats, but I still stay away from political parties," Bunin wrote in the early 1910s. He said he realised now that the working class had become a force powerful enough to "overcome the whole of Western Europe," but warned against the possible negative effect of the Russian workers' lack of organisation, the one thing that made them different from their Western counterparts. He criticised the Russian intelligentsia for being ignorant of the common people's life, and spoke of a tragic schism between "the cultured people and the uncultured masses."

In December 1910 Bunin and Muromtseva made another journey to the Middle East, then visited Ceylon; this four-month trip inspired such stories as "Brothers" (Братья) and "The Tsar of Tsars City" (Город царя царей). On his return to Odessa in April 1911, Bunin wrote "Waters Aplenty" (Воды многие), a travel diary, much lauded after its publication in 1926. In 1912 the novel Dry Valley (Суходол) came out, his second major piece of semi-autobiographical fiction, concerning the dire state of the Russian rural community. Again it left the literary critics divided: social democrats praised its stark honesty, many others were appalled with the author's negativism.

Bunin and Muromtseva spent three winters (1912–1914) with Gorky on the island of Capri, where they met with Fyodor Shalyapin and Leonid Andreev, among others. In Russia the couple divided their time mainly between Moscow and a Bunin family estate at Glotovo village nearby Oryol; it was there that they spent the first couple years of World War I. Dogged by anxieties concerning Russia's future, Bunin was still working hard. In the winter of 1914–1915 he finished a new volume of prose and verse entitled The Chalice of Life (Чаша жизни), published in early 1915 to wide acclaim (including high praise from the French poet Rene Ghil). The same year saw the publication of The Gentleman from San Francisco (Господин из Сан-Франциско), arguably the best-known of Bunin's short stories, which was translated into English by D. H. Lawrence. Bunin was a productive translator himself. After Longfellow's The Song of Hiawatha (1898), he did translations of Byron, Tennyson, Musset and François Coppée.

During the war years, Bunin completed the preparation of a six-volume edition of his Collected Works, which was published by Adolph Marks in 1915. Throughout this time Bunin kept aloof from contemporary literary debates. "I did not belong to any literary school; I was neither a decadent, nor a symbolist nor a romantic, nor a naturalist. Of literary circles I frequented only a few," he commented later. By the spring of 1916, overcome by pessimism, Bunin all but stopped writing, complaining to his nephew, N.A. Pusheshnikov, of how insignificant he felt as a writer and how depressed he was for being unable to do more than be horrified at the millions of deaths being caused by the War.

In May 1917 the Bunins moved to Glotovo and stayed there until autumn. In October the couple returned to Moscow to stay with Vera's parents. Life in the city was dangerous (residents had to guard their own homes, maintaining nightly vigils) but Bunin still visited publishers and took part in the meetings of the Sreda and The Art circles. While dismissive of Ivan Goremykin (the 1914–1916 Russian Government Premier), he criticised opposition figures like Pavel Milyukov as "false defenders of the Russian people". In April 1917 he severed all ties with the pro-revolutionary Gorky, causing a rift which would never be healed. On 21 May 1918, Bunin and Muromtseva obtained the official permission to leave Moscow for Kiev, then continued their journey through to Odessa. By 1919 Bunin was working for the Volunteer Army as the editor of the cultural section of the anti-Bolshevik newspaper Iuzhnoe Slovo. On 26 January 1920, the couple boarded the last French ship in Odessa and soon were in Constantinople.