quality:corruption, structural:reformatting
1972–1974: Move to Island Records

In 1972, Bob Marley signed with CBS Records in London and embarked on a UK tour with soul singer Johnny Nash. While in London the Wailers asked their road manager Brent Clarke to introduce them to Chris Blackwell, who had licensed some of their Coxsone releases for his Island Records. The Wailers intended to discuss the royalties associated with these releases; instead, the meeting resulted in the offer of an advance of £4,000 to record an album. Since Jimmy Cliff, Island's top reggae star, had recently left the label, Blackwell was primed for a replacement. In Marley, Blackwell recognised the elements needed to snare the rock audience: "I was dealing with rock music, which was really rebel music. I felt that would really be the way to break Jamaican music. But you needed someone who could be that image. When Bob walked in he really was that image." The Wailers returned to Jamaica to record at Harry J's in Kingston, which resulted in the album Catch a Fire.

Primarily recorded on an eight-track, Catch a Fire marked the first time a reggae band had access to a state-of-the-art studio and were accorded the same care as their rock 'n' roll peers. Blackwell desired to create "more of a drifting, hypnotic-type feel than a reggae rhythm", and restructured Marley's mixes and arrangements. Marley travelled to London to supervise Blackwell's overdubbing of the album at Island Studios, which included tempering the mix from the bass-heavy sound of Jamaican music and omitting two tracks.

The Wailers' first album for Island, Catch a Fire, was released worldwide in April 1973, packaged like a rock record with a unique Zippo lighter lift-top. Initially selling 14,000 units, it received a positive critical reception. It was followed later that year by the album Burnin', which included the song " I Shot the Sheriff ". Eric Clapton was given the album by his guitarist George Terry in the hope that he would enjoy it. Clapton was impressed and chose to record a cover version of "I Shot the Sheriff", which became his first US hit since " Layla " two years earlier and reached number 1 on the Billboard Hot 100 on 14 September 1974. Many Jamaicans were not keen on the new reggae sound on Catch a Fire, but the Trenchtown style of Burnin found fans across both reggae and rock audiences.

During this period, Blackwell gifted his Kingston residence and company headquarters at 56 Hope Road (then known as Island House) to Marley. Housing Tuff Gong Studios, the property became not only Marley's office but also his home.

The Wailers were scheduled to open 17 shows in the US for Sly and the Family Stone. After four shows, the band was fired because they were more popular than the acts they were opening for. The Wailers disbanded in 1974, with each of the three main members pursuing a solo career.